Study of the promotion mechanism of the photocatalytic performance and stability of the Ag@AgCl/g-C3N4 composite under visible light
Bu, Yuyu1; Chen, Zhuoyuan1; Feng, Chang2; Li, Weibing2; Chen, ZY (reprint author), Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, 7 Nanhai Rd, Qingdao 266071, Peoples R China.
2014
发表期刊RSC ADVANCES
卷号4期号:72页码:38124-38132
文章类型Article
摘要The Ag@AgCl/g-C3N4 composite was prepared by in situ fabricating Ag@AgCl on the surface of g-C3N4 using deposition-precipitation and subsequently photo-assisted reduction. Both the photocatalytic degradation performance and the photocatalytic degradation stability of the Ag@AgCl/g-C3N4 composite are significantly improved compared to g-C3N4 and Ag@AgCl composite. The Ag@AgCl/g-C3N4 composite can completely degrade RhB in 20 min under the illumination of visible light (lambda > 420 nm). The Ag@AgCl/g-C3N4 composite can increase the light absorption intensity in the visible light region due to the surface plasmon resonance effect of Ag, resulting in a significant increase of the yields of the photogenerated electrons and holes. An effective heterojunction electric field was formed on the interface between g-C3N4 and Ag@AgCl, which significantly strengthened the separation efficiency of the photogenerated electrons and holes, leading to a significant promotion of the photocatalytic degradation performance.
学科领域Chemistry
DOI10.1039/c4ra04957h
收录类别SCI
语种英语
WOS记录号WOS:000341455200024
引用统计
被引频次:31[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.qdio.ac.cn/handle/337002/23888
专题海洋环境腐蚀与生物污损重点实验室
通讯作者Chen, ZY (reprint author), Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, 7 Nanhai Rd, Qingdao 266071, Peoples R China.
作者单位1.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Peoples R China
2.Qingdao Univ Sci & Technol, Sch Environm & Safety Engn, Qingdao 266042, Peoples R China
第一作者单位中国科学院海洋研究所
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GB/T 7714
Bu, Yuyu,Chen, Zhuoyuan,Feng, Chang,et al. Study of the promotion mechanism of the photocatalytic performance and stability of the Ag@AgCl/g-C3N4 composite under visible light[J]. RSC ADVANCES,2014,4(72):38124-38132.
APA Bu, Yuyu,Chen, Zhuoyuan,Feng, Chang,Li, Weibing,&Chen, ZY .(2014).Study of the promotion mechanism of the photocatalytic performance and stability of the Ag@AgCl/g-C3N4 composite under visible light.RSC ADVANCES,4(72),38124-38132.
MLA Bu, Yuyu,et al."Study of the promotion mechanism of the photocatalytic performance and stability of the Ag@AgCl/g-C3N4 composite under visible light".RSC ADVANCES 4.72(2014):38124-38132.
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