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Study of the promotion mechanism of the photocatalytic performance and stability of the Ag@AgCl/g-C3N4 composite under visible light | |
Bu, Yuyu1; Chen, Zhuoyuan1; Feng, Chang2; Li, Weibing2; Chen, ZY (reprint author), Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, 7 Nanhai Rd, Qingdao 266071, Peoples R China. | |
2014 | |
发表期刊 | RSC ADVANCES |
卷号 | 4期号:72页码:38124-38132 |
文章类型 | Article |
摘要 | The Ag@AgCl/g-C3N4 composite was prepared by in situ fabricating Ag@AgCl on the surface of g-C3N4 using deposition-precipitation and subsequently photo-assisted reduction. Both the photocatalytic degradation performance and the photocatalytic degradation stability of the Ag@AgCl/g-C3N4 composite are significantly improved compared to g-C3N4 and Ag@AgCl composite. The Ag@AgCl/g-C3N4 composite can completely degrade RhB in 20 min under the illumination of visible light (lambda > 420 nm). The Ag@AgCl/g-C3N4 composite can increase the light absorption intensity in the visible light region due to the surface plasmon resonance effect of Ag, resulting in a significant increase of the yields of the photogenerated electrons and holes. An effective heterojunction electric field was formed on the interface between g-C3N4 and Ag@AgCl, which significantly strengthened the separation efficiency of the photogenerated electrons and holes, leading to a significant promotion of the photocatalytic degradation performance. |
学科领域 | Chemistry |
DOI | 10.1039/c4ra04957h |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000341455200024 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.qdio.ac.cn/handle/337002/23888 |
专题 | 海洋环境腐蚀与生物污损重点实验室 |
通讯作者 | Chen, ZY (reprint author), Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, 7 Nanhai Rd, Qingdao 266071, Peoples R China. |
作者单位 | 1.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Peoples R China 2.Qingdao Univ Sci & Technol, Sch Environm & Safety Engn, Qingdao 266042, Peoples R China |
第一作者单位 | 中国科学院海洋研究所 |
推荐引用方式 GB/T 7714 | Bu, Yuyu,Chen, Zhuoyuan,Feng, Chang,et al. Study of the promotion mechanism of the photocatalytic performance and stability of the Ag@AgCl/g-C3N4 composite under visible light[J]. RSC ADVANCES,2014,4(72):38124-38132. |
APA | Bu, Yuyu,Chen, Zhuoyuan,Feng, Chang,Li, Weibing,&Chen, ZY .(2014).Study of the promotion mechanism of the photocatalytic performance and stability of the Ag@AgCl/g-C3N4 composite under visible light.RSC ADVANCES,4(72),38124-38132. |
MLA | Bu, Yuyu,et al."Study of the promotion mechanism of the photocatalytic performance and stability of the Ag@AgCl/g-C3N4 composite under visible light".RSC ADVANCES 4.72(2014):38124-38132. |
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