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S vacancy in MoS2 nanosheets induces H2O cleavage: a new era for 2D nanozyme
Wang, Jin1,2,3; Ren, Wenyu1,3; Wang, Yi1,2,3; Zhang, Dun1,2,3; Wang, Yu4; Ju, Peng5; Dou, Kunpeng6
2023-09-21
Source PublicationRESEARCH ON CHEMICAL INTERMEDIATES
ISSN0922-6168
Volume49Issue:12Pages:10
Corresponding AuthorWang, Yi(wangyi@qdio.ac.cn)
AbstractNanozyme is a promising approach in treating pollution in drinking water sources. 2D MoS2 nanosheets, with abundant active sites and Lewis acid sites, exhibit outstanding peroxidase-like activity. Verified by density functional calculation, S vacancies in 2D MoS2 nanosheets can cleavage H2O to yield H+ and .OH. The spontaneous generation of acid environment and oxygen free radicals enables 2D MoS2 nanosheets to be effectively exploited in the depuration of polluted water, creating a new era for multifunctional nanozymes.
KeywordMoS2 Nanozyme Peroxidase-like activity S vacancy DFT calculations
DOI10.1007/s11164-023-05135-y
Indexed BySCI
Language英语
Funding ProjectNatural Science Foundation of China[42176047] ; Second Batch of Postdoctoral Funding in Qingdao in 2022 ; 2022 Special Research Assistant Program of the Chinese Academy of Science ; 73rd batch of general support from China Postdoctoral Science Foundation
WOS Research AreaChemistry
WOS SubjectChemistry, Multidisciplinary
WOS IDWOS:001071123100004
PublisherSPRINGER
WOS KeywordPEROXIDASE-LIKE ACTIVITY ; REDUCTION ; ENZYMES
Citation statistics
Cited Times:1[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.qdio.ac.cn/handle/337002/181535
Collection海洋环境腐蚀与生物污损重点实验室
Corresponding AuthorWang, Yi
Affiliation1.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100039, Peoples R China
3.Pilot Natl Lab Marine Sci & Technol, Open Studio Marine Corros & Protect, Qingdao 266237, Peoples R China
4.Soochow Univ, Coll Pharmaceut Sci, Suzhou 215123, Peoples R China
5.Minist Nat Resources, Inst Oceanog 1, Marine Bioresource & Environm Res Ctr, Key Lab Marine Ecoenvironm Sci & Technol, Qingdao 266061, Peoples R China
6.Ocean Univ China, Coll Informat Sci & Engn, Qingdao 266100, Peoples R China
First Author AffilicationInstitute of Oceanology, Chinese Academy of Sciences
Corresponding Author AffilicationInstitute of Oceanology, Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Wang, Jin,Ren, Wenyu,Wang, Yi,et al. S vacancy in MoS2 nanosheets induces H2O cleavage: a new era for 2D nanozyme[J]. RESEARCH ON CHEMICAL INTERMEDIATES,2023,49(12):10.
APA Wang, Jin.,Ren, Wenyu.,Wang, Yi.,Zhang, Dun.,Wang, Yu.,...&Dou, Kunpeng.(2023).S vacancy in MoS2 nanosheets induces H2O cleavage: a new era for 2D nanozyme.RESEARCH ON CHEMICAL INTERMEDIATES,49(12),10.
MLA Wang, Jin,et al."S vacancy in MoS2 nanosheets induces H2O cleavage: a new era for 2D nanozyme".RESEARCH ON CHEMICAL INTERMEDIATES 49.12(2023):10.
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