Institutional Repository of Key Laboratory of Marine Environmental Corrosion and Bio-fouling, IOCAS
Self-healing performance and corrosion resistance of graphene oxide-mesoporous silicon layer-nanosphere structure coating under marine alternating hydrostatic pressure | |
Wang, Wei1,2,3,6; Wang, Hongliang4; Zhao, Jie2,6![]() ![]() | |
2019-04-01 | |
Source Publication | CHEMICAL ENGINEERING JOURNAL
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ISSN | 1385-8947 |
Volume | 361Pages:792-804 |
Corresponding Author | Wang, Wei(wangwei8038@ouc.edu.cn) ; Song, Liying(songliying0520@163.com) ; Li, Weihua(liweihua@qdio.ac.cn) |
Abstract | Alternating hydrostatic pressure (AHP) is the main cause of the marine coating failure of deep-sea tools and equipment. Herein, we synthesized a novel nanostructure, namely, graphene oxide-mesoporous silicon dioxide layer-nanosphere structure loaded with tannic acid (GSLNTA), as a self-healing coating additive. The anticorrosion and anti-AHP performance and the self-healing capability of GSLNTA coating were evaluated through electrochemical impedance spectroscopy, field emission scanning electron microscopy, Fourier-transform infrared spectroscopy, and alternating current scanning electrochemical microscopy (AC-SECM). Results showed that the nanolayer structure of GSLNTA effectively inhibited corrosion mass transmission under simulated deepsea AHP. The nanospheres of GSLNTA released inhibitors to form a ferric tannate film on the exposed metal surface under AHP. The nanolayer and nanosphere of GSLNTA self-healing coating exerted a synergistic effect on anti-corrosion and anti-AHP performance and blocked corrosion factor transmission and coating failure in deepsea applications. AC-SECM revealed the advantages of local impedance complementation of different electrochemical parameters (vertical bar Z vertical bar and -phase) to monitor the self-healing of coatings with GSLNTA. This work also investigated the self-healing performance of alkyd varnish coating embedded with synthetic GSLNTA in protecting steel surfaces. Self-healing materials have an "active healing" capability to prolong the life of organic coatings after unwanted external damage in deep-sea environments. |
Keyword | Self-healing coating Deep-sea Alternating hydrostatic pressure Corrosion Alternating current scanning electrochemical microscopy |
DOI | 10.1016/j.cej.2018.12.124 |
Indexed By | SCI |
Language | 英语 |
Funding Project | National Science Fund for Distinguished Young Scholars[51525903] ; National Natural Science Foundation of China[51709253] ; National Natural Science Foundation of China[51601188] ; Opening Foundation of State Key Laboratory of Marine Resource Utilization in South China Sea[2018005] ; applied Basic Research Programs of Qingdao[17-1-1-98-jch] ; AoShan Talents Cultivation Program ; Qingdao National Laboratory for Marine Science and Technology[2017ASTCP-OS09] ; Excellent Middle-Aged and Youth Scientist Award Foundation of Shandong Province[BS2014CL005] ; National Science Fund for Distinguished Young Scholars[51525903] ; National Natural Science Foundation of China[51709253] ; National Natural Science Foundation of China[51601188] ; Opening Foundation of State Key Laboratory of Marine Resource Utilization in South China Sea[2018005] ; Applied Basic Research Programs of Qingdao[17-1-1-98-jch] ; AoShan Talents Cultivation Program ; Qingdao National Laboratory for Marine Science and Technology[2017ASTCP-OS09] ; Excellent Middle-Aged and Youth Scientist Award Foundation of Shandong Province[BS2014CL005] |
WOS Research Area | Engineering |
WOS Subject | Engineering, Environmental ; Engineering, Chemical |
WOS ID | WOS:000457096400078 |
Publisher | ELSEVIER SCIENCE SA |
Citation statistics | |
Document Type | 期刊论文 |
Identifier | http://ir.qdio.ac.cn/handle/337002/160823 |
Collection | 海洋环境腐蚀与与生物污损重点实验室 |
Corresponding Author | Wang, Wei; Song, Liying; Li, Weihua |
Affiliation | 1.Ocean Univ China, Inst Mat Sci & Engn, 238 Songling Rd, Qingdao 266100, Peoples R China 2.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, 7 Nanhai Rd, Qingdao 266071, Peoples R China 3.Hainan Univ, Key Lab Marine Resource Utilizat South China Sea, Haikou 570228, Hainan, Peoples R China 4.State Ocean Adm, Natl Deep Sea Ctr, Qingdao 266237, Peoples R China 5.Sun Yat Sen Univ, Sch Chem Engn & Technol, Zhuhai 519082, Peoples R China 6.Qingdao Natl Lab Marine Sci & Technol, 1 Wenhai Rd, Qingdao 266237, Peoples R China |
First Author Affilication | Institute of Oceanology, Chinese Academy of Sciences |
Corresponding Author Affilication | Institute of Oceanology, Chinese Academy of Sciences |
Recommended Citation GB/T 7714 | Wang, Wei,Wang, Hongliang,Zhao, Jie,et al. Self-healing performance and corrosion resistance of graphene oxide-mesoporous silicon layer-nanosphere structure coating under marine alternating hydrostatic pressure[J]. CHEMICAL ENGINEERING JOURNAL,2019,361:792-804. |
APA | Wang, Wei.,Wang, Hongliang.,Zhao, Jie.,Wang, Xin.,Xiong, Chuansheng.,...&Li, Weihua.(2019).Self-healing performance and corrosion resistance of graphene oxide-mesoporous silicon layer-nanosphere structure coating under marine alternating hydrostatic pressure.CHEMICAL ENGINEERING JOURNAL,361,792-804. |
MLA | Wang, Wei,et al."Self-healing performance and corrosion resistance of graphene oxide-mesoporous silicon layer-nanosphere structure coating under marine alternating hydrostatic pressure".CHEMICAL ENGINEERING JOURNAL 361(2019):792-804. |
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