| Spatial distributions and sources of heavy metals in sediments of the Changjiang Estuary and its adjacent coastal areas based on mercury, lead and strontium isotopic compositions | |
Cheng, Yaxin1; Zhang, Rui1,2,3,4,5,6 ; Li, Tiegang7,8,9; Zhang, Fan10; Russell, James4; Guan, Minglei1; Han, Qi11; Zhou, Yurou10; Xiao, Xin10; Wang, Xiqi10
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| 2019-03-01 | |
| 发表期刊 | CATENA
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| ISSN | 0341-8162 |
| 卷号 | 174页码:154-163 |
| 通讯作者 | Zhang, Rui(rzhang_838@163.com) ; Li, Tiegang(tgli@fio.org.cn) |
| 摘要 | The distribution, source and fate of the heavy metals mercury (Hg) and lead (Pb) in surface sediments from the East China Sea (ECS) were studied using mercury, lead and strontium (Sr) isotopic ratios. Hydrodynamic circulation and the sedimentary depositional process within the ECS were the dominant factors controlling the distribution and fate of heavy metals, referring from relationships of heavy metals (Hg and Pb) concentrations and total organic carbon (TOC) and clay contents. Spatial variations in Hg isotopic compositions (delta Hg-220) were observed in the ECS, with delta Hg-202 ranging from -1.86 to -0.83 parts per thousand and Delta Hg-199 ranging from -0.07 to +0.26 parts per thousand. The high delta Hg-202 values and relatively negative Delta Hg-199 values in estuarine and inner shelf sites indicated that the riverine inputs from Changjiang River played an important role in delivering Hg to ECS. In contrast, Hg isotopic signatures in outer shelf sediments had relatively low delta Hg-202 and positive Delta Hg-199, implying that atmospheric Hg deposition could be a relatively dominant source for Hg. Using these Hg isotope compositions, the source attributions of sediments in ECS were estimated based on a triple mixing model, suggesting that river-dominated inputs, discharging pollutants from industrial sources, and atmospheric deposition could dominate in the occurrence and fate of Hg in surface sediments of ECS. Moreover, the results of Pb and Sr isotopic ratios in surface sediment samples and potential sources showed that the Pb accumulated in the ECS was mainly from background and anthropogenic sources, with the contribution rates of 45% and 55%, respectively. |
| 关键词 | Mercury Lead Isotopic tracer Source identification East China Sea Anthropogenic inputs |
| DOI | 10.1016/j.catena.2018.10.039 |
| 收录类别 | SCI |
| 语种 | 英语 |
| 资助项目 | National Natural Science Foundation of China[41406055] ; National Natural Science Foundation of China[41230959] ; National Natural Science Foundation of China[41476043] ; National Natural Science Foundation of China[41506106] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDA11030104] ; National Program on Global Change and Air-Sea Interaction[GASI-GEOGE-06-02] ; National Program on Global Change and Air-Sea Interaction[GASI-GEOGE-04] ; International Postdoctoral Exchange Fellowship Program[20160073] ; Natural Science Foundation of Jiangsu Province[BK20170451] ; Natural Science Foundation of Jiangsu Province[BE2016701] ; Six Talent Peaks Project in Jiangsu Province[JNHB-143] ; Natural Science Foundation of Lianyungang City[SH1506] ; Natural Science Foundation of Lianyungang City[CN1510] ; National Natural Science Foundation of China[41406055] ; National Natural Science Foundation of China[41230959] ; National Natural Science Foundation of China[41476043] ; National Natural Science Foundation of China[41506106] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDA11030104] ; National Program on Global Change and Air-Sea Interaction[GASI-GEOGE-06-02] ; National Program on Global Change and Air-Sea Interaction[GASI-GEOGE-04] ; International Postdoctoral Exchange Fellowship Program[20160073] ; Natural Science Foundation of Jiangsu Province[BK20170451] ; Natural Science Foundation of Jiangsu Province[BE2016701] ; Six Talent Peaks Project in Jiangsu Province[JNHB-143] ; Natural Science Foundation of Lianyungang City[SH1506] ; Natural Science Foundation of Lianyungang City[CN1510] |
| WOS研究方向 | Geology ; Agriculture ; Water Resources |
| WOS类目 | Geosciences, Multidisciplinary ; Soil Science ; Water Resources |
| WOS记录号 | WOS:000456754600014 |
| 出版者 | ELSEVIER SCIENCE BV |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | http://ir.qdio.ac.cn/handle/337002/160680 |
| 专题 | 海洋地质与环境重点实验室 |
| 通讯作者 | Zhang, Rui; Li, Tiegang |
| 作者单位 | 1.Huaihai Inst Technol, Sch Geodesy & Geomat Engn, Lianyungang 222005, Jiangsu, Peoples R China 2.Huaihai Inst Technol, Jiangsu Key Lab Marine Bioresources & Environm, Lianyungang 222005, Jiangsu, Peoples R China 3.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Geol & Environm, Qingdao 266071, Peoples R China 4.Brown Univ, Dept Earth Environm & Planetary Sci, Providence, RI 02912 USA 5.Huaihai Inst Technol, Coinnovat Ctr Jiangsu Marine Bioind Technol, Lianyungang 222005, Jiangsu, Peoples R China 6.Jiangsu Marine Resources Dev Res Inst, Lianyungang 222005, Jiangsu, Peoples R China 7.State Ocean Adm, Inst Oceanog 1, Qingdao 266061, Shandong, Peoples R China 8.Qingdao Natl Lab Marine Sci & Technol, Lab Marine Geol, Qingdao 266061, Peoples R China 9.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 10.Huaihai Inst Technol, Dept Chem Engn, Lianyungang 222005, Jiangsu, Peoples R China 11.China Univ Geosci, Sch Ocean Sci, Beijing 100083, Peoples R China |
| 通讯作者单位 | 中国科学院海洋研究所 |
| 推荐引用方式 GB/T 7714 | Cheng, Yaxin,Zhang, Rui,Li, Tiegang,et al. Spatial distributions and sources of heavy metals in sediments of the Changjiang Estuary and its adjacent coastal areas based on mercury, lead and strontium isotopic compositions[J]. CATENA,2019,174:154-163. |
| APA | Cheng, Yaxin.,Zhang, Rui.,Li, Tiegang.,Zhang, Fan.,Russell, James.,...&Wang, Xiqi.(2019).Spatial distributions and sources of heavy metals in sediments of the Changjiang Estuary and its adjacent coastal areas based on mercury, lead and strontium isotopic compositions.CATENA,174,154-163. |
| MLA | Cheng, Yaxin,et al."Spatial distributions and sources of heavy metals in sediments of the Changjiang Estuary and its adjacent coastal areas based on mercury, lead and strontium isotopic compositions".CATENA 174(2019):154-163. |
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