| In situ Raman Quantitative Detection of the Cold Seep Vents and Fluids in the Chemosynthetic Communities in the South China Sea | |
Du, Zengfeng1,2; Zhang, Xin1,2,3; Luan, Zhendong1,2; Wang, Minxiao1,2; Xi, Shichuan1,3; Li, Lianfu1,3; Wang, Bing1,3; Cao, Lei1 ; Lian, Chao1; Li, Chaolun1,2,3; Yan, Jun1
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| 2018-07-01 | |
| 发表期刊 | GEOCHEMISTRY GEOPHYSICS GEOSYSTEMS
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| ISSN | 1525-2027 |
| 卷号 | 19期号:7页码:2049-2061 |
| 通讯作者 | Zhang, Xin(xzhang@qdio.ac.cn) |
| 摘要 | Based on the previously developed deep-sea hybrid Raman insertion probe for cold seeps, the in situ detection of a cold seep vent and geochemistry analysis of fluids in chemosynthetic communities were conducted at the Formosa Ridge in the northern South China Sea. Three different methods were used to measure the components of the fluids erupting from the cold seep vent. The in situ Raman spectra of the cold seep fluids indicated the presence of gaseous CH4, C3H8, and H2S. The results indicate that the gases at this site are of biogenic origin; however, the presence of C3H8 suggests that thermogenic methane should not be excluded. The conclusion is also supported by the results of gas chromatography and stable carbon isotope analysis. More significantly, we found that the concentration of SO42- decreases with increasing depth, while the concentrations of CH4 and S-8 increase in fluids in chemosynthetic communities, but without H2S. This finding indicates that the methane is oxidized by sulfate and that elemental sulfur is formed. This process usually occurs in marine sediments as the anaerobic oxidation of methane. Overall, the findings in this work provide a new insight into the geochemical analysis of cold seep fluids and in situ evidence of the oxidation of methane in the chemosynthetic communities near cold seeps. |
| 关键词 | Raman spectroscopy in situ detection cold seep fluids chemosynthetic communities |
| DOI | 10.1029/2018GC007496 |
| 收录类别 | SCI |
| 语种 | 英语 |
| 资助项目 | National Natural Science Foundation of China[41576104] ; Key Research Program of Frontier Sciences, CAS[QYZDB-SSW-DQC004] ; Strategic Priority Research Program, CAS[XDA11040301] ; Strategic Priority Research Program, CAS[XDA11030301] ; Open Research Project of the National Major Science & Technology Infrastructure (RV KEXUE)[NMSTI-KEXUE2017K01] ; NSFC-Shandong Joint Fund for Marine Science Research Centers[U1606401] ; National Key R&D Program of China[2016YFC0302103] ; Taishan Scholar Project Funding[tspd20161007] ; National Natural Science Foundation of China[41576104] ; Key Research Program of Frontier Sciences, CAS[QYZDB-SSW-DQC004] ; Strategic Priority Research Program, CAS[XDA11040301] ; Strategic Priority Research Program, CAS[XDA11030301] ; Open Research Project of the National Major Science & Technology Infrastructure (RV KEXUE)[NMSTI-KEXUE2017K01] ; NSFC-Shandong Joint Fund for Marine Science Research Centers[U1606401] ; National Key R&D Program of China[2016YFC0302103] ; Taishan Scholar Project Funding[tspd20161007] |
| WOS研究方向 | Geochemistry & Geophysics |
| WOS类目 | Geochemistry & Geophysics |
| WOS记录号 | WOS:000443389300009 |
| 出版者 | AMER GEOPHYSICAL UNION |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | http://ir.qdio.ac.cn/handle/337002/160022 |
| 专题 | 海洋地质与环境重点实验室 深海极端环境与生命过程研究中心 |
| 通讯作者 | Zhang, Xin |
| 作者单位 | 1.Chinese Acad Sci, Inst Oceanol, Ctr Deep Sea Res, CAS Key Lab Marine Geol & Environm, Qingdao, Peoples R China 2.Qingdao Natl Lab Marine Sci & Technol, Lab Marine Geol, Qingdao, Peoples R China 3.Univ Chinese Acad Sci, Beijing, Peoples R China |
| 第一作者单位 | 深海极端环境与生命过程研究中心 |
| 通讯作者单位 | 深海极端环境与生命过程研究中心 |
| 推荐引用方式 GB/T 7714 | Du, Zengfeng,Zhang, Xin,Luan, Zhendong,et al. In situ Raman Quantitative Detection of the Cold Seep Vents and Fluids in the Chemosynthetic Communities in the South China Sea[J]. GEOCHEMISTRY GEOPHYSICS GEOSYSTEMS,2018,19(7):2049-2061. |
| APA | Du, Zengfeng.,Zhang, Xin.,Luan, Zhendong.,Wang, Minxiao.,Xi, Shichuan.,...&Yan, Jun.(2018).In situ Raman Quantitative Detection of the Cold Seep Vents and Fluids in the Chemosynthetic Communities in the South China Sea.GEOCHEMISTRY GEOPHYSICS GEOSYSTEMS,19(7),2049-2061. |
| MLA | Du, Zengfeng,et al."In situ Raman Quantitative Detection of the Cold Seep Vents and Fluids in the Chemosynthetic Communities in the South China Sea".GEOCHEMISTRY GEOPHYSICS GEOSYSTEMS 19.7(2018):2049-2061. |
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| 文件名称/大小 | 文献类型 | 版本类型 | 开放类型 | 使用许可 | ||
| In situ Raman Quanti（3553KB） | 期刊论文 | 出版稿 | 限制开放 | CC BY-NC-SA | 浏览 | |
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