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| Water-soluble nitrogen and phosphorus in aerosols and dry deposition in Jiaozhou Bay, North China: Deposition velocities, origins and biogeochemical implications | |
Xing, Jianwei1,2,3 ; Song, Jinming1,2,3; Yuan, Huamao1,2,3; Wang, Qidong1,2,3; Li, Xuegang1,2,3; Li, Ning1,2,3; Duan, Liqin1,2,3; Qu, Baoxiao1,2,3
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| 2018-07-15 | |
| 发表期刊 | ATMOSPHERIC RESEARCH
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| ISSN | 0169-8095 |
| 卷号 | 207页码:90-99 |
| 摘要 | To probe the deposition velocities (V-d), fluxes, origins and biogeochemical significance of atmospheric dry deposition (ADD) of nutrients in coastal waters, aerosol and dry deposition samples were collected in Jiaozhou Bay (JZB) from June 2015 to May 2016. We measured water-soluble inorganic nitrogen (WSIN; including ammonium (NH4-N), nitrate (NO3-N) and nitrite (NO2-N)), organic nitrogen (WSON), inorganic phosphorus (WSIP; including reactive phosphate (PO4-P)) and organic phosphorus (WSOP) for all samples. The concentrations of aerosol N species were comparatively higher than those in other aquatic ecosystems worldwide. Although WSIN and WSIP represented relatively large percentages of species, WSON (similar to 16%) and WSOP (similar to 35%) cannot be ignored in aerosols. The dry deposition fluxes for NH4-N, NO3-N, NO2-N, WSON, PO4-P and WSOP were 29.4, 29.9, 0.058, 15.4, 0.099 and 0.165 mmol m(-2) yr(-1), respectively, with apparent seasonal variations. The average annual Vd values of NH4-N, NO3-N, NO2-N, WSON, PO4-P and WSOP were indirectly calculated as 0.17 +/- 0.11, 0.35 +/- 0.20, 0.34 +/- 0.25, 0.30 +/- 0.22, 0.43 +/- 0.28 and 0.91 +/- 0.60 cm s(-1), respectively. The considerable differences between the percentages of corresponding nutrient concentrations and ADD fluxes were mainly attributed to Vd variations. Anthropogenic emissions were the most common source of WSON and WSIN based on a correlation analysis. WSIP was highly correlated with WSOP, suggesting that they may share similar sources. Additionally, the long-range transport of natural and anthropogenic pollutants, especially the air-masses originating from the northwest direction, exerted greater effects than local emissions on aerosol N and P species in JZB based on an air mass backward trajectory analysis. The increasing ADD flux may have non negligible biogeochemical effects on JZB by increasing primary productivity and altering the nutrient structure due to the high WSIN/WSIP ratio. |
| 关键词 | Water-soluble nitrogen Water-soluble phosphorus Dry deposition velocities Origins New productivity Jiaozhou Bay (JZB) |
| DOI | 10.1016/j.atrnosres.2018.03.001 |
| 收录类别 | SCI |
| 语种 | 英语 |
| 资助项目 | National Natural Science Foundation of China (NSFC)[41676068] ; Qingdao National Laboratory for Marine Science and Technology[2015ASTP-OS13] ; Postdoctoral Applied Research Project of Qingdao ; National Program on Key Basic Research Project of China (973 Program)[2015CB452902] ; National Program on Key Basic Research Project of China (973 Program)[2015CB452901] ; Shandong Province for Marine Science Research Centers[U1606404] ; National Natural Science Foundation[U1606404] ; National Natural Science Foundation[U1606404] ; Shandong Province for Marine Science Research Centers[U1606404] ; National Program on Key Basic Research Project of China (973 Program)[2015CB452901] ; National Program on Key Basic Research Project of China (973 Program)[2015CB452902] ; Postdoctoral Applied Research Project of Qingdao ; Qingdao National Laboratory for Marine Science and Technology[2015ASTP-OS13] ; National Natural Science Foundation of China (NSFC)[41676068] |
| WOS研究方向 | Meteorology & Atmospheric Sciences |
| WOS类目 | Meteorology & Atmospheric Sciences |
| WOS记录号 | WOS:000430901800007 |
| 出版者 | ELSEVIER SCIENCE INC |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 版本 | 出版稿 |
| 条目标识符 | http://ir.qdio.ac.cn/handle/337002/158980 |
| 专题 | 海洋生态与环境科学重点实验室 |
| 通讯作者 | Song, Jinming |
| 作者单位 | 1.Chinese Acad Sci, Inst Oceanol, CAS Key Lab Marine Ecol & Environm Sci, Qingdao 266071, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Qingdao Natl Lab Marine Sci & Technol, Funct Lab Marine Ecol & Environm Sci, Qingdao 266237, Peoples R China |
| 第一作者单位 | 海洋生态与环境科学重点实验室 |
| 通讯作者单位 | 海洋生态与环境科学重点实验室 |
| 推荐引用方式 GB/T 7714 | Xing, Jianwei,Song, Jinming,Yuan, Huamao,et al. Water-soluble nitrogen and phosphorus in aerosols and dry deposition in Jiaozhou Bay, North China: Deposition velocities, origins and biogeochemical implications[J]. ATMOSPHERIC RESEARCH,2018,207:90-99. |
| APA | Xing, Jianwei.,Song, Jinming.,Yuan, Huamao.,Wang, Qidong.,Li, Xuegang.,...&Qu, Baoxiao.(2018).Water-soluble nitrogen and phosphorus in aerosols and dry deposition in Jiaozhou Bay, North China: Deposition velocities, origins and biogeochemical implications.ATMOSPHERIC RESEARCH,207,90-99. |
| MLA | Xing, Jianwei,et al."Water-soluble nitrogen and phosphorus in aerosols and dry deposition in Jiaozhou Bay, North China: Deposition velocities, origins and biogeochemical implications".ATMOSPHERIC RESEARCH 207(2018):90-99. |
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