Long term corrosion estimation of carbon steel, titanium and its alloy in backfill material of compacted bentonite for nuclear waste repository
Zhang, Qichao1,2,6; Zheng, Min1,2; Huang, Yanliang1,6; Kunte, Hans Joerg3; Wang, Xiutong1,6; Liu, Yuemiao4; Zheng, Chuanbo5
2019-03-01
发表期刊SCIENTIFIC REPORTS
ISSN2045-2322
卷号9页码:18
通讯作者Huang, Yanliang(hyl@qdio.ac.cn)
摘要The container of high-level radioactive waste (HLRW) being in deep geological disposal, the backfill material is needed to serve as the second defense for HLRW and the highly compacted bentonite is generally selected. As the time goes, the underground water will infiltrate the backfill, causing the corrosion of materials for the building of containers in the formed electrolyte. Carbon steel, titanium and its alloy are the potential candidate materials for the fabrication of HLRW containers. The current investigation aims at assessing the safety of HLRW container in deep geological disposal for hundreds of thousands of years and facilitating the material selection for future container fabrication by estimating their corrosion behavior in compacted bentonite with a series of moisture content at different temperatures through electrochemical methods including open circuit potential (OCP), electrochemical impedance spectroscopy (EIS) and potentiodynamic polarization curve (PC) measurements. The corrosion rates were estimated for a carbon steel, a pure titanium and a titanium alloy in compacted Gaomiaozi Bentonite infiltrated with simulated underground water in Beishan area of China over an expected disposal period up to 10(6) years respectively, showing that titanium and its alloy are more reliable materials for building HLRW containers than carbon steel.
DOI10.1038/s41598-019-39751-9
收录类别SCI
语种英语
资助项目National Natural Science Foundation of China[51471160] ; National Natural Science Foundation of China[51471160]
WOS研究方向Science & Technology - Other Topics
WOS类目Multidisciplinary Sciences
WOS记录号WOS:000459983900001
出版者NATURE PUBLISHING GROUP
引用统计
被引频次:20[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.qdio.ac.cn/handle/337002/155238
专题海洋环境腐蚀与生物污损重点实验室
通讯作者Huang, Yanliang
作者单位1.Chinese Acad Sci, Inst Oceanol, Qingdao 266071, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Bundesanstalt Mat Forsch & Prufung, D-12205 Berlin, Germany
4.Beijing Res Inst Uranium Geol, Beijing 100029, Peoples R China
5.Jiangsu Univ Sci & Technol, Sch Mat Sci & Engn, Zhenjiang 212003, Jiangsu, Peoples R China
6.Qingdao Natl Lab Marine Sci & Technol, Open Studio Marine Corros & Protect, Qingdao 266237, Peoples R China
第一作者单位中国科学院海洋研究所
通讯作者单位中国科学院海洋研究所
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Zhang, Qichao,Zheng, Min,Huang, Yanliang,et al. Long term corrosion estimation of carbon steel, titanium and its alloy in backfill material of compacted bentonite for nuclear waste repository[J]. SCIENTIFIC REPORTS,2019,9:18.
APA Zhang, Qichao.,Zheng, Min.,Huang, Yanliang.,Kunte, Hans Joerg.,Wang, Xiutong.,...&Zheng, Chuanbo.(2019).Long term corrosion estimation of carbon steel, titanium and its alloy in backfill material of compacted bentonite for nuclear waste repository.SCIENTIFIC REPORTS,9,18.
MLA Zhang, Qichao,et al."Long term corrosion estimation of carbon steel, titanium and its alloy in backfill material of compacted bentonite for nuclear waste repository".SCIENTIFIC REPORTS 9(2019):18.
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