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Understanding Complex Electrochemical Impedance Spectroscopy in Corrosion Systems Using in-situ Synchrotron Radiation Grazing Incidence X-ray Diffraction
Alam, Muhammad Tanzirul1; Chan, Emilyn Wai Lyn2; De Marco, Roland1,2,3; Huang, Yanliang4; Bailey, Stuart2
2016-09-01
发表期刊ELECTROANALYSIS
卷号28期号:9页码:2166-2170
文章类型Article
摘要The difficulty in interpreting electrochemical impedance spectroscopy (EIS) data has limited the potential of the method despite its utility as an electrochemical method for studies of electrode reactions and interfacial structures. Taking the test case of the carbon dioxide corrosion of carbon steel, in-situ synchrotron radiation grazing incidence X-ray diffraction (SR-GIXRD) has been demonstrated to be a powerful technique for validating and understanding the interfacial structures associated with complex EIS data. Carbon dioxide corrosion was found to occur in several steps, which may only be surmised by EIS, but the use of SR-GIXRD in conjunction with EIS has enabled the establishment of a link between EIS time constants and structural changes associated with the evolution of corrosion products with time. By comparison to previous studies by the authors and others in this field, this communication provides the first direct experimental evidence linking SR-GIXRD surface compositional data to otherwise indistinctive EIS time constants.
关键词Carbon Dioxide Corrosion Carbon Steel Impedance Synchrotron Radiation Chukanovite
DOI10.1002/elan.201600137
收录类别SCI
语种英语
WOS记录号WOS:000386932800033
引用统计
被引频次:3[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
版本出版稿
条目标识符http://ir.qdio.ac.cn/handle/337002/135944
专题海洋腐蚀与防护研究发展中心
作者单位1.Univ Sunshine Coast, Fac Sci Hlth Educ & Engn, B1-59,90 Sippy Downs Dr, Sippy Downs, Qld 4556, Australia
2.Curtin Univ, Dept Chem, GPO Box U1987, Perth, WA 6109, Australia
3.Univ Queensland, Sch Chem & Mol Biosci, Brisbane, Qld 4072, Australia
4.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Peoples R China
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Alam, Muhammad Tanzirul,Chan, Emilyn Wai Lyn,De Marco, Roland,et al. Understanding Complex Electrochemical Impedance Spectroscopy in Corrosion Systems Using in-situ Synchrotron Radiation Grazing Incidence X-ray Diffraction[J]. ELECTROANALYSIS,2016,28(9):2166-2170.
APA Alam, Muhammad Tanzirul,Chan, Emilyn Wai Lyn,De Marco, Roland,Huang, Yanliang,&Bailey, Stuart.(2016).Understanding Complex Electrochemical Impedance Spectroscopy in Corrosion Systems Using in-situ Synchrotron Radiation Grazing Incidence X-ray Diffraction.ELECTROANALYSIS,28(9),2166-2170.
MLA Alam, Muhammad Tanzirul,et al."Understanding Complex Electrochemical Impedance Spectroscopy in Corrosion Systems Using in-situ Synchrotron Radiation Grazing Incidence X-ray Diffraction".ELECTROANALYSIS 28.9(2016):2166-2170.
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