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Fabrication of g-C3N4/Au/CdZnS Z-scheme photocatalyst to enhance photocatalysis performance
Ma, Xiumin1; Jiang, Quantong1; Guo, Weimin2; Zheng, Meng1; Xu, Weichen1; Ma, Fubin1; Hou, Baorong1
2016
发表期刊RSC ADVANCES
卷号6期号:34页码:28263-28269
文章类型Article
摘要In this study, a sandwich-structured C3N4/Au/CdZnS photocatalyst with Au nanoparticles sandwiched between C3N4 and CdZnS was fabricated. The results showed that there was a 6.3 mmol g(-1) increase of hydrogen production for C3N4/Au/CdZnS photocatalyst compared to C3N4/CdZnS in 4 h. The photoinduced I-t curve, electrochemical impedance spectrum (EIS), photogenerated electron lifetime and photoluminescence spectra showed that the photocatalytic ability of the composite was enhanced by anchoring Au as the electron transfer mediator between C3N4 and CdZnS through the Z-scheme charge-carrier transfer mechanism. Au functioned as an electron transition mediator, which could induce a combination between photogenerated electrons and holes in the CdZnS and C3N4, respectively. These photogenerated holes of CdZnS can be involved in the S2-/SO32- oxidation process and the electrons from the C3N4 surface might be involved in the water to hydrogen reduction reaction, thus enhancing the photocatalysis performance of C3N4/Au/CdZnS photocatalyst.
DOI10.1039/c5ra27429j
收录类别SCI
语种英语
WOS记录号WOS:000372610200015
引用统计
文献类型期刊论文
条目标识符http://ir.qdio.ac.cn/handle/337002/126213
专题海洋腐蚀与防护研究发展中心
作者单位1.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, 7 Nanhai Rd, Qingdao 266071, Peoples R China
2.Luoyang Ship Mat Res Inst, State Key Marine Corros & Protect, Qingdao 266101, Peoples R China
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Ma, Xiumin,Jiang, Quantong,Guo, Weimin,et al. Fabrication of g-C3N4/Au/CdZnS Z-scheme photocatalyst to enhance photocatalysis performance[J]. RSC ADVANCES,2016,6(34):28263-28269.
APA Ma, Xiumin.,Jiang, Quantong.,Guo, Weimin.,Zheng, Meng.,Xu, Weichen.,...&Hou, Baorong.(2016).Fabrication of g-C3N4/Au/CdZnS Z-scheme photocatalyst to enhance photocatalysis performance.RSC ADVANCES,6(34),28263-28269.
MLA Ma, Xiumin,et al."Fabrication of g-C3N4/Au/CdZnS Z-scheme photocatalyst to enhance photocatalysis performance".RSC ADVANCES 6.34(2016):28263-28269.
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